Photocatalytic reductive sulfonylation and 1,2-alkyl migration cascades of vinyl cyclobutanols: A synthesis of beta-sulfonated cyclopentanones

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초록

A photoredox strategy to access beta-sulfonated cyclopentanones from the reaction of vinyl cyclobutanols with sulfonyl chlorides is described. This reaction employs the inexpensive and easily accessible sulfonyl chlorides as a sulfonyl radical source. The present synthetic protocol is a convenient way to prepare beta-sulfonated cyclopentanones.

키워드

beta-sulfonated cyclopentanonesphotoredox processsemipinacol-type rearrangementsulfonyl chloridesvinyl cyclobutanolsVISIBLE-LIGHT PHOTOREDOXASYMMETRIC-SYNTHESISRING EXPANSIONKETO ACIDSMETAL-FREECYCLIZATIONSEQUENCESTETRAHYDROQUINOLINESALKENESOXIDATION
제목
Photocatalytic reductive sulfonylation and 1,2-alkyl migration cascades of vinyl cyclobutanols: A synthesis of beta-sulfonated cyclopentanones
저자
Kim, Joo HeeKim, Dae Young
DOI
10.1080/00397911.2019.1692223
발행일
2020-01-17
유형
Article
저널명
Synthetic Communications
50
2
페이지
207 ~ 216